Adding of other materials ( organic colors) to the salt solution would disturb the growing of the crystals.
For alum type Me(I)Me(III)SO4 x 18 H2O, exchange the Me( III) in this case Al to Cr, Fe, V, Mn, Co, and others. Me(I) can be K and to higher Alkali metals like Rb or Cs.Also NH4+ or Tl can be used.