Maybe you could have one solution in a beaker (e.g.) and maybe spray a certain volume of the other solution into it. That way, you have droplets. The only problem is that you won't have an accurate way of saying "this is the particle size." Instead, it'll have to be things like "tiny," etc. For larger sizes, you could use apparati that spray with large droplets, and at the extremity, just pour the entire solution in at once.